UniSysCat: Publications 2020

Publications 2020

Life as we don't (yet) know it, N. Budisa in Art as we don’t know it (Hrsg.: Berger, E.; Kasperi Mäki-Reinikka; Kira O’Reilly; Sederholm, H., ), Aalto University Publication Series, 2020, 0–0, ISBN: 9789526088228
Ultralight covalent organic framework/graphene aerogels with hierarchical porosity, C. Li, J. Yang, P. Pachfule, S. Li, M. Y. Ye, J. Schmidt, A. Thomas, Nature Communications 2020, 11, 10.1038/s41467-020-18427-3
Revisiting the Intriguing Electronic Features of the BeOBeC Carbyne and Some Isomers: A Quantum‐Chemical Assessment, J. Li, C. Geng, T. Weiske, M. Zhou, J. Li, H. Schwarz, Angewandte Chemie International Edition 2020, 10.1002/anie.202007990
Probing the Structure of [NiFeSe] Hydrogenase with QM/MM Computations, S. Moubarak, N. Elghobashi-Meinhardt, D. Tombolelli, M. A. Mroginski, Applied Sciences 2020, 10, 781–0, 10.3390/app10030781
Absorption and Emission Spectroscopic Investigation of the Thermal Dynamics of the Archaerhodopsin 3 Based Fluorescent Voltage Sensor Archon2, A. Penzkofer, A. Silapetere, P. Hegemann, International Journal of Molecular Sciences 2020, 21, 6576–0, 10.3390/ijms21186576
Dual Photoisomerization on Distinct Potential Energy Surfaces in a UV-Absorbing Rhodopsin, Y. Hontani, M. Broser, M. Luck, J. Weißenborn, M. Kloz, P. Hegemann, J. T. M. Kennis, Journal of the American Chemical Society 2020, 142, 11464–11473, 10.1021/jacs.0c03229
Caught in the H : Crystal Structure and Spectroscopy Reveal a Sulfur Bound to the Active Site of an O ‐stable State of [FeFe] Hydrogenase, P. Rodríguez‐Maciá, L. M. Galle, R. Bjornsson, C. Lorent, I. Zebger, Y. Yoda, S. P. Cramer, S. DeBeer, I. Span, J. A. Birrell, Angewandte Chemie International Edition 2020, 10.1002/anie.202005208
A Local Hybrid Functional with Wide Applicability and Good Balance between (De)Localization and Left–Right Correlation, M. Haasler, T. M. Maier, R. Grotjahn, S. Gückel, A. V. Arbuznikov, M. Kaupp, Journal of Chemical Theory and Computation 2020, 16, 5645–5657, 10.1021/acs.jctc.0c00498
Phosphoglycolate salvage in a chemolithoautotroph using the Calvin cycle, N. J. Claassens, G. Scarinci, A. Fischer, A. I. Flamholz, W. Newell, S. Frielingsdorf, O. Lenz, A. Bar-Even, Proceedings of the National Academy of Sciences 2020, 117, 22452–22461, 10.1073/pnas.2012288117
Dihydrogen‐Driven NADPH Recycling in Imine Reduction and P450‐Catalyzed Oxidations Mediated by an Engineered O ‐Tolerant Hydrogenase, J. Preissler, H. A. Reeve, T. Zhu, J. Nicholson, K. Urata, L. Lauterbach, L. L. Wong, K. A. Vincent, O. Lenz, ChemCatChem 2020, 10.1002/cctc.202000763
The large subunit of the regulatory [NiFe]-hydrogenase from – a minimal hydrogenase?, G. Caserta, C. Lorent, A. Ciaccafava, M. Keck, R. Breglia, C. Greco, C. Limberg, P. Hildebrandt, S. P. Cramer, I. Zebger, O. Lenz, Chemical Science 2020, 11, 5453–5465, 10.1039/D0SC01369B
A membrane‐bound [NiFe]‐hydrogenase large subunit precursor whose C‐terminal extension is not essential for cofactor incorporation but guarantees optimal maturation, S. Hartmann, S. Frielingsdorf, G. Caserta, O. Lenz, MicrobiologyOpen 2020, 9, 1197–1206, 10.1002/mbo3.1029
Bringing biocatalytic deuteration into the toolbox of asymmetric isotopic labelling techniques, J. S. Rowbotham, M. A. Ramirez, O. Lenz, H. A. Reeve, K. A. Vincent, Nature Communications 2020, 11, 10.1038/s41467-020-15310-z
[FeFe]-hydrogenase maturation: H-cluster assembly intermediates tracked by electron paramagnetic resonance, infrared, and X-ray absorption spectroscopy, B. Németh, M. Senger, H. J. Redman, P. Ceccaldi, J. Broderick, A. Magnuson, S. T. Stripp, M. Haumann, G. Berggren, JBIC Journal of Biological Inorganic Chemistry 2020, 25, 777–788, 10.1007/s00775-020-01799-8
Operando Raman spectroscopy tracks oxidation-state changes in an amorphous Co oxide material for electrocatalysis of the oxygen evolution reaction, C. Pasquini, L. D’Amario, I. Zaharieva, H. Dau, The Journal of Chemical Physics 2020, 152, 194202–0, 10.1063/5.0006306
A synthetic manganese–calcium cluster similar to the catalyst of Photosystem II: challenges for biomimetic water oxidation, Y. Mousazade, M. R. Mohammadi, R. Bagheri, R. Bikas, P. Chernev, Z. Song, T. Lis, M. Siczek, N. Noshiranzadeh, S. Mebs, H. Dau, I. Zaharieva, M. M. Najafpour, Dalton Transactions 2020, 49, 5597–5605, 10.1039/d0dt00536c
Exploring the Limits of Self-Repair in Cobalt Oxide Films for Electrocatalytic Water Oxidation, M. R. Mohammadi, S. Loos, P. Chernev, C. Pasquini, I. Zaharieva, D. González-Flores, P. Kubella, K. Klingan, R. D. L. Smith, H. Dau, ACS Catalysis 2020, 10, 7990–7999, 10.1021/acscatal.0c01944
Electrocatalytic CO Reduction on CuO Nanocubes: Tracking the Evolution of Chemical State, Geometric Structure, and Catalytic Selectivity using Operando Spectroscopy, T. Möller, F. Scholten, T. N. Thanh, I. Sinev, J. Timoshenko, X. Wang, Z. Jovanov, M. Gliech, B. Roldan Cuenya, A. S. Varela, P. Strasser, Angewandte Chemie 2020, 10.1002/ange.202007136
Synthesis of New Aza‐ and Thia‐Crown Ether Based Amino Acids, T. Schneider, N. Brüssow, A. Yuvanc, N. Budisa, ChemistrySelect 2020, 5, 2854–2857, 10.1002/slct.202000122
Xenobiology: A Journey towards Parallel Life Forms, N. Budisa, V. Kubyshkin, M. Schmidt, ChemBioChem 2020, 21, 2228–2231, 10.1002/cbic.202000141
Phage capsid nanoparticles with defined ligand arrangement block influenza virus entry, D. Lauster, S. Klenk, K. Ludwig, S. Nojoumi, S. Behren, L. Adam, M. Stadtmüller, S. Saenger, S. Zimmler, K. Hönzke, L. Yao, U. Hoffmann, M. Bardua, A. Hamann, M. Witzenrath, L. E. Sander, T. Wolff, A. C. Hocke, S. Hippenstiel, S. De Carlo, J. Neudecker, K. Osterrieder, N. Budisa, R. R. Netz, C. Böttcher, S. Liese, A. Herrmann, C. P. R. Hackenberger, Nature Nanotechnology 2020, 15, 373–379, 10.1038/s41565-020-0660-2
Discovery and Characterization of a New Cold-Active Protease From an Extremophilic Bacterium via Comparative Genome Analysis and in vitro Expression, A. Perfumo, G. J. Freiherr von Sass, E. L. Nordmann, N. Budisa, D. Wagner, Frontiers in Microbiology 2020, 11, 10.3389/fmicb.2020.00881
Catalytic dioxygen reduction mediated by a tetranuclear cobalt complex supported on a stannoxane core, A. Chandra, S. Mebs, S. Kundu, U. Kuhlmann, P. Hildebrandt, H. Dau, K. Ray, Dalton Transactions 2020, 49, 6065–6073, 10.1039/d0dt00475h
Overcoming Chemical Inertness under Ambient Conditions: A Critical View on Recent Developments in Ammonia Synthesis via Electrochemical N Reduction by Asking Five Questions, Q. Qin, M. Oschatz, ChemElectroChem 2020, 7, 878–889, 10.1002/celc.201901970
Influence of Local Environments in Pores of Different Size on the Catalytic Liquid-Phase Oxidation of -Glucose by Au Nanoparticles Supported on Nanoporous Carbon, M. Perovic, N. V. Tarakina, J. P. Hofmann, M. Oschatz, ACS Applied Nano Materials 2020, 3, 7695–7703, 10.1021/acsanm.0c01299
A Simple Nickel Catalyst Enabling an ‐Selective Alkyne Semihydrogenation, N. O. Thiel, B. Kaewmee, T. Tran Ngoc, J. F. Teichert, Chemistry – A European Journal 2020, 26, 1597–1603, 10.1002/chem.201903850
Impact of Nanomorphology on Surface Doping of Organic Semiconductors: The Pentacene–C F Interface, F. Silvestri, M. J. Prieto, A. Babuji, L. C. Tănase, L. de Souza Caldas, O. Solomeshch, T. Schmidt, C. Ocal, E. Barrena, ACS Applied Materials & Interfaces 2020, 12, 25444–25452, 10.1021/acsami.0c05583
The role of in situ generated morphological motifs and Cu(i) species in C2+ product selectivity during CO2 pulsed electroreduction, R. M. Arán-Ais, F. Scholten, S. Kunze, R. Rizo, B. Roldan Cuenya, Nature Energy 2020, 5, 317–325, 10.1038/s41560-020-0594-9
Iron and manganese oxo complexes, oxo wall and beyond, V. A. Larson, B. Battistella, K. Ray, N. Lehnert, W. Nam, Nature Reviews Chemistry 2020, 4, 404–419, 10.1038/s41570-020-0197-9
Stoichiometric Formation of an Oxoiron(IV) Complex by a Soluble Methane Monooxygenase Type Activation of O at an Iron(II)-Cyclam Center, D. Kass, T. Corona, K. Warm, B. Braun-Cula, U. Kuhlmann, E. Bill, S. Mebs, M. Swart, H. Dau, M. Haumann, P. Hildebrandt, K. Ray, Journal of the American Chemical Society 2020, 142, 5924–5928, 10.1021/jacs.9b13756
Enhancing Tris(pyrazolyl)borate‐Based Models of Cysteine/Cysteamine Dioxygenases through Steric Effects: Increased Reactivities, Full Product Characterization and Hints to Initial Superoxide Formation, L. Müller, S. Hoof, M. Keck, C. Herwig, C. Limberg, Chemistry – A European Journal 2020, 26, 11851–11861, 10.1002/chem.202001818
Assessment of the manganese cluster’s oxidation state via photoactivation of photosystem II microcrystals, M. H. Cheah, M. Zhang, D. Shevela, F. Mamedov, A. Zouni, J. Messinger, Proceedings of the National Academy of Sciences 2020, 117, 141–145, 10.1073/pnas.1915879117
Counter‐Intuitive Gas‐Phase Reactivities of [V ] and [V O] towards CO Reduction: Insight from Electronic Structure Calculations, J. Li, C. Geng, T. Weiske, H. Schwarz, Angewandte Chemie International Edition 2020, 59, 12308–12314, 10.1002/anie.202001223
Overcoming limitations in dual photoredox/nickel-catalysed C–N cross-couplings due to catalyst deactivation, S. Gisbertz, S. Reischauer, B. Pieber, Nature Catalysis 2020, 3, 611–620, 10.1038/s41929-020-0473-6
Heterogeneous Photocatalysis in Organic Synthesis, S. Gisbertz, B. Pieber, ChemPhotoChem 2020, 4, 456–475, 10.1002/cptc.202000014
Evidence for Photocatalyst Involvement in Oxidative Additions of Nickel-Catalyzed Carboxylate -Arylations, J. A. Malik, A. Madani, B. Pieber, P. H. Seeberger, Journal of the American Chemical Society 2020, 142, 11042–11049, 10.1021/jacs.0c02848
An oscillatory plug flow photoreactor facilitates semi-heterogeneous dual nickel/carbon nitride photocatalytic C–N couplings, C. Rosso, S. Gisbertz, J. D. Williams, H. P. L. Gemoets, W. Debrouwer, B. Pieber, C. O. Kappe, Reaction Chemistry & Engineering 2020, 5, 597–604, 10.1039/d0re00036a
Spectroscopic investigations under whole-cell conditions provide new insight into the metal hydride chemistry of [FeFe]-hydrogenase, L. S. Mészáros, P. Ceccaldi, M. Lorenzi, H. J. Redman, E. Pfitzner, J. Heberle, M. Senger, S. T. Stripp, G. Berggren, Chemical Science 2020, 11, 4608–4617, 10.1039/D0SC00512F
Electrochemical Biosensors Employing Natural and Artificial Heme Peroxidases on Semiconductors, B. Neumann, U. Wollenberger, Sensors 2020, 20, 3692–0, 10.3390/s20133692
Vibrational characterization of a diiron bridging hydride complex – a model for hydrogen catalysis, L. B. Gee, V. Pelmenschikov, H. Wang, N. Mishra, Y. C. Liu, Y. Yoda, K. Tamasaku, M. H. Chiang, S. P. Cramer, Chemical Science 2020, 11, 5487–5493, 10.1039/d0sc01290d
On the Crucial Role of Isolated Electronic States in the Thermal Reaction of ReC with Dihydrogen, J. Li, C. Geng, T. Weiske, H. Schwarz, Angewandte Chemie International Edition 2020, 59, 9370–9376, 10.1002/anie.202001599
Shedding Light on Proton and Electron Dynamics in [FeFe] Hydrogenases, C. Lorent, S. Katz, J. Duan, C. J. Kulka, G. Caserta, C. Teutloff, S. Yadav, U. P. Apfel, M. Winkler, T. Happe, M. Horch, I. Zebger, Journal of the American Chemical Society 2020, 142, 5493–5497, 10.1021/jacs.9b13075
Imaging electrochemically synthesized Cu2O cubes and their morphological evolution under conditions relevant to CO2 electroreduction, R. M. Arán-Ais, R. Rizo, P. Grosse, G. Algara-Siller, K. Dembélé, M. Plodinec, T. Lunkenbein, S. W. Chee, B. Roldan Cuenya, Nature Communications 2020, 11, 10.1038/s41467-020-17220-6
In-situ structure and catalytic mechanism of NiFe and CoFe layered double hydroxides during oxygen evolution, F. Dionigi, Z. Zeng, I. Sinev, T. Merzdorf, S. Deshpande, M. B. Lopez, S. Kunze, I. Zegkinoglou, H. Sarodnik, D. Fan, A. Bergmann, J. Drnec, J. F. d. Araujo, M. Gliech, D. Teschner, J. Zhu, W. X. Li, J. Greeley, B. Roldan Cuenya, P. Strasser, Nature Communications 2020, 11, 10.1038/s41467-020-16237-1
Cryo-EM structures reveal intricate Fe-S cluster arrangement and charging in Rhodobacter capsulatus formate dehydrogenase, C. Radon, G. Mittelstädt, B. R. Duffus, J. Bürger, T. Hartmann, T. Mielke, C. Teutloff, S. Leimkühler, P. Wendler, Nature Communications 2020, 11, 10.1038/s41467-020-15614-0
Transition metal-based catalysts for the electrochemical CO₂ reduction: from atoms and molecules to nanostructured materials, F. Franco, C. Rettenmaier, H. S. Jeon, B. Roldan Cuenya, Chemical Society Reviews 2020, 49, 6884–6946, 10.1039/D0CS00835D
In-cell architecture of an actively transcribing-translating expressome, F. J. O’Reilly, L. Xue, A. Graziadei, L. Sinn, S. Lenz, D. Tegunov, C. Blötz, N. Singh, W. J. H. Hagen, P. Cramer, J. Stülke, J. Mahamid, J. Rappsilber, Science 2020, 369, 554–557, 10.1126/science.abb3758
On the Borate-Catalyzed Electrochemical Reduction of Phosphine Oxide: A Computational Study, R. Edler von Zander, P. Saalfrank, The Journal of Physical Chemistry A 2020, 124, 10239–10245, 10.1021/acs.jpca.0c07805
Reversible Water-Induced Phase Changes of Cobalt Oxide Nanoparticles, D. Hein, G. Wartner, A. Bergmann, M. Bernal, B. Roldan Cuenya, R. Seidel, ACS Nano 2020, 14, 15450–15457, 10.1021/acsnano.0c06066
Enhanced Formic Acid Oxidation over SnO₂ -decorated Pd Nanocubes, C. Rettenmaier, R. M. Arán-Ais, J. Timoshenko, R. Rizo, H. S. Jeon, S. Kühl, S. W. Chee, A. Bergmann, B. Roldan Cuenya, ACS Catalysis 2020, 10, 14540–14551, 10.1021/acscatal.0c03212
On the Activity/Selectivity and Phase Stability of Thermally Grown Copper Oxides during the Electrocatalytic Reduction of CO₂, J. J. Velasco-Vélez, C. H. Chuang, D. Gao, Q. Zhu, D. Ivanov, H. S. Jeon, R. Arrigo, R. V. Mom, E. Stotz, H. L. Wu, T. E. Jones, B. Roldan Cuenya, A. Knop-Gericke, R. Schlögl, ACS Catalysis 2020, 10, 11510–11518, 10.1021/acscatal.0c03484
Operando NRIXS and XAFS Investigation of Segregation Phenomena in Fe‐Cu and Fe‐Ag Nanoparticle Catalysts during CO₂ Electroreduction, S. Kunze, P. Grosse, M. Bernal Lopez, I. Sinev, I. Zegkinoglou, H. Mistry, J. Timoshenko, M. Y. Hu, J. Zhao, E. E. Alp, S. W. Chee, B. Roldan Cuenya, Angewandte Chemie International Edition 2020, 59, 22667–22674, 10.1002/anie.202010535
Growth Dynamics and Processes Governing the Stability of Electrodeposited Size-Controlled Cubic Cu Catalysts, P. Grosse, A. Yoon, C. Rettenmaier, S. W. Chee, B. Roldan Cuenya, The Journal of Physical Chemistry C 2020, 124, 26908–26915, 10.1021/acs.jpcc.0c09105
In Vitro Assembly as a Tool to Investigate Catalytic Intermediates of [NiFe]-Hydrogenase, G. Caserta, C. Lorent, V. Pelmenschikov, J. Schoknecht, Y. Yoda, P. Hildebrandt, S. P. Cramer, I. Zebger, O. Lenz, ACS Catalysis 2020, 10, 13890–13894, 10.1021/acscatal.0c04079
High-Frequency Fe–H and Fe–H2 Modes in a trans-Fe(η2-H2)(H) Complex: A Speed Record for Nuclear Resonance Vibrational Spectroscopy, M. H. Chiang, V. Pelmenschikov, L. B. Gee, Y. C. Liu, C. C. Hsieh, H. Wang, Y. Yoda, H. Matsuura, L. Li, S. P. Cramer, Inorganic Chemistry 2020, 60, 555–559, 10.1021/acs.inorgchem.0c03006
Cobalt‐Exchanged Poly(Heptazine Imides) as Transition Metal–N Electrocatalysts for the Oxygen Evolution Reaction, M. Ye, S. Li, X. Zhao, N. V. Tarakina, C. Teutloff, W. Y. Chow, R. Bittl, A. Thomas, Advanced Materials 2020, 32, 1903942–0, 10.1002/adma.201903942
Atomic Layer Deposition of ZnO on Mesoporous Silica: Insights into Growth Behavior of ZnO via In-Situ Thermogravimetric Analysis, P. Ingale, K. Knemeyer, M. Piernavieja Hermida, R. Naumann d’Alnoncourt, A. Thomas, F. Rosowski, Nanomaterials 2020, 10, 981–0, 10.3390/nano10050981
Synthesis of Vinylene-Linked Covalent Organic Frameworks from Acetonitrile: Combining Cyclotrimerization and Aldol Condensation in One Pot, A. Acharjya, L. Longworth-Dunbar, J. Roeser, P. Pachfule, A. Thomas, Journal of the American Chemical Society 2020, 142, 14033–14038, 10.1021/jacs.0c04570
A composite of clay, cement, and wood as natural support material for the immobilization of commercial titania (P25, P90, PC500, C-TiO2) towards photocatalytic phenol degradation, L. Morjène, M. Tasbihi, M. Schwarze, R. Schomäcker, F. Aloulou, M. Seffen, Water Science and Technology 2020, 81, 1882–1893, 10.2166/wst.2020.244
Pd nanoparticles confined in mesoporous N-doped carbon silica supports: a synergistic effect between catalyst and support, R. L. Oliveira, J. Kerstien, R. Schomäcker, A. Thomas, Catalysis Science & Technology 2020, 10, 1385–1394, 10.1039/c9cy01920k
Surface Hopping Dynamics for Azobenzene Photoisomerization: Effects of Packing Density on Surfaces, Fluorination, and Excitation Wavelength, C. Rietze, E. Titov, G. Granucci, P. Saalfrank, The Journal of Physical Chemistry C 2020, 124, 26287–26295, 10.1021/acs.jpcc.0c08052
Multiomics Analysis Provides Insight into the Laboratory Evolution of toward the Metabolic Usage of Fluorinated Indoles, F. Agostini, L. Sinn, D. Petras, C. J. Schipp, V. Kubyshkin, A. A. Berger, P. C. Dorrestein, J. Rappsilber, N. Budisa, B. Koksch, ACS Central Science 2020, 7, 81–92, 10.1021/acscentsci.0c00679
Cryo-EM structures of holo condensin reveal a subunit flip-flop mechanism, B. G. Lee, F. Merkel, M. Allegretti, M. Hassler, C. Cawood, L. Lecomte, F. J. O’Reilly, L. R. Sinn, P. Gutierrez-Escribano, M. Kschonsak, S. Bravo, T. Nakane, J. Rappsilber, L. Aragon, M. Beck, J. Löwe, C. H. Haering, Nature structural & molecular biology 2020, 27, 743–751, 10.1038/s41594-020-0457-x
The structure of human thyroglobulin, F. Coscia, A. Taler-Verčič, V. T. Chang, L. Sinn, F. J. O’Reilly, T. Izoré, M. Renko, I. Berger, J. Rappsilber, D. Turk, J. Löwe, Nature 2020, 578, 627–630, 10.1038/s41586-020-1995-4
Combining free energy calculations with tailored enzyme activity assays to elucidate substrate binding of a phospho-lysine phosphatase, A. Hauser, S. Hwang, H. Sun, C. P. R. Hackenberger, Chemical Science 2020, 11, 12655–12661, 10.1039/D0SC03930F
Solution Structure of the Detergent–Photosystem II Core Complex Investigated by Small-Angle Scattering Techniques, M. Golub, R. Hussein, M. Ibrahim, M. Hecht, D. C. F. Wieland, A. Martel, B. Machado, A. Zouni, J. Pieper, The Journal of Physical Chemistry B 2020, 124, 8583–8592, 10.1021/acs.jpcb.0c07169
Untangling the sequence of events during the S → S transition in photosystem II and implications for the water oxidation mechanism, M. Ibrahim, T. Fransson, R. Chatterjee, M. H. Cheah, R. Hussein, L. Lassalle, K. D. Sutherlin, I. D. Young, F. D. Fuller, S. Gul, I. S. Kim, P. S. Simon, C. de Lichtenberg, P. Chernev, I. Bogacz, C. C. Pham, A. M. Orville, N. Saichek, T. Northen, A. Batyuk, S. Carbajo, R. Alonso-Mori, K. Tono, S. Owada, A. Bhowmick, R. Bolotovsky, D. Mendez, N. W. Moriarty, J. M. Holton, H. Dobbek, A. S. Brewster, P. D. Adams, N. K. Sauter, U. Bergmann, A. Zouni, J. Messinger, J. Kern, V. K. Yachandra, J. Yano, Proceedings of the National Academy of Sciences 2020, 117, 12624–12635, 10.1073/pnas.2000529117
Structural basis of light‐harvesting in the photosystem II core complex, F. Müh, A. Zouni, Protein Science 2020, 29, 1090–1119, 10.1002/pro.3841
pH‐Dependent Protonation of Surface Carboxylate Groups in PsbO Enables Local Buffering and Triggers Structural Changes, L. Gerland, D. Friedrich, L. Hopf, E. J. Donovan, A. Wallmann, N. Erdmann, A. Diehl, M. Bommer, K. Buzar, M. Ibrahim, P. Schmieder, H. Dobbek, A. Zouni, A. Bondar, H. Dau, H. Oschkinat, ChemBioChem 2020, 21, 1597–1604, 10.1002/cbic.201900739
Strongly Reducing (Diarylamino)benzene-Based Covalent Organic Framework for Metal-Free Visible Light Photocatalytic H O Generation, C. Krishnaraj, H. Sekhar Jena, L. Bourda, A. Laemont, P. Pachfule, J. Roeser, C. V. Chandran, S. Borgmans, S. M. J. Rogge, K. Leus, C. V. Stevens, J. A. Martens, V. Van Speybroeck, E. Breynaert, A. Thomas, P. Van Der Voort, Journal of the American Chemical Society 2020, 142, 20107–20116, 10.1021/jacs.0c09684
Electrochemical N Reduction to Ammonia Using Single Au/Fe Atoms Supported on Nitrogen-Doped Porous Carbon, S. K. Sahoo, J. Heske, M. Antonietti, Q. Qin, M. Oschatz, T. D. Kühne, ACS Applied Energy Materials 2020, 3, 10061–10069, 10.1021/acsaem.0c01740
From Molecular Precursors to Nanoparticles—Tailoring the Adsorption Properties of Porous Carbon Materials by Controlled Chemical Functionalization, M. Perovic, Q. Qin, M. Oschatz, Advanced Functional Materials 2020, 30, 1908371–0, 10.1002/adfm.201908371
Immobilization of Gold‐on‐Carbon Catalysts Onto Perfluorocarbon Emulsion Droplets to Promote Oxygen Delivery in Aqueous Phase ‐Glucose Oxidation, M. Perovic, L. Zeininger, M. Oschatz, ChemCatChem 2020, 13, 196–201, 10.1002/cctc.202001590
Surface Conditions That Constrain Alkane Oxidation on Perovskites, G. Koch, M. Hävecker, D. Teschner, S. J. Carey, Y. Wang, P. Kube, W. Hetaba, T. Lunkenbein, G. Auffermann, O. Timpe, F. Rosowski, R. Schlögl, A. Trunschke, ACS Catalysis 2020, 10, 7007–7020, 10.1021/acscatal.0c01289
Towards Experimental Handbooks in Catalysis, A. Trunschke, G. Bellini, M. Boniface, S. J. Carey, J. Dong, E. Erdem, L. Foppa, W. Frandsen, M. Geske, L. M. Ghiringhelli, F. Girgsdies, R. Hanna, M. Hashagen, M. Hävecker, G. Huff, A. Knop-Gericke, G. Koch, P. Kraus, J. Kröhnert, P. Kube, S. Lohr, T. Lunkenbein, L. Masliuk, R. Naumann d’Alnoncourt, T. Omojola, C. Pratsch, S. Richter, C. Rohner, F. Rosowski, F. Rüther, M. Scheffler, R. Schlögl, A. Tarasov, D. Teschner, O. Timpe, P. Trunschke, Y. Wang, S. Wrabetz, Topics in Catalysis 2020, 63, 1683–1699, 10.1007/s11244-020-01380-2
Promoting Photocatalytic Hydrogen Evolution Activity of Graphitic Carbon Nitride with Hole‐Transfer Agents, A. Indra, R. Beltrán‐Suito, M. Müller, R. P. Sivasankaran, M. Schwarze, A. Acharjya, B. Pradhan, J. Hofkens, A. Brückner, A. Thomas, P. W. Menezes, M. Driess, ChemSusChem 2020, 14, 306–312, 10.1002/cssc.202002500
Synthesis and Coordination Ability of a Donor‐Stabilised Bis‐Phosphinidene, T. J. Hadlington, A. Kostenko, M. Driess, Chemistry – A European Journal 2020, 27, 2476–2482, 10.1002/chem.202004300
Crystalline Copper Selenide as a Reliable Non‐Noble Electro(pre)catalyst for Overall Water Splitting, B. Chakraborty, R. Beltrán‐Suito, V. Hlukhyy, J. Schmidt, P. W. Menezes, M. Driess, ChemSusChem 2020, 13, 3222–3229, 10.1002/cssc.202000445
Improved chemical water oxidation with Zn in the tetrahedral site of spinel-type ZnCo2O4 nanostructure, B. Chakraborty, A. Indra, P. V. Menezes, M. Driess, P. W. Menezes, Materials Today Chemistry 2020, 15, 100226–0, 10.1016/j.mtchem.2019.100226
A soft molecular 2Fe–2As precursor approach to the synthesis of nanostructured FeAs for efficient electrocatalytic water oxidation, R. Beltrán-Suito, V. Forstner, J. N. Hausmann, S. Mebs, J. Schmidt, I. Zaharieva, K. Laun, I. Zebger, H. Dau, P. W. Menezes, M. Driess, Chemical Science 2020, 11, 11834–11842, 10.1039/D0SC04384B
Understanding the formation of bulk- and surface-active layered (oxy)hydroxides for water oxidation starting from a cobalt selenite precursor, J. N. Hausmann, S. Mebs, K. Laun, I. Zebger, H. Dau, P. W. Menezes, M. Driess, Energy & Environmental Science 2020, 13, 3607–3619, 10.1039/D0EE01912G
Bis(silylene)‐Stabilized Monovalent Nitrogen Complexes, S. Yao, T. Szilvási, Y. Xiong, C. Lorent, A. Ruzicka, M. Driess, Angewandte Chemie International Edition 2020, 59, 22043–22047, 10.1002/anie.202011598
Detecting structural transformation of cobalt phosphonate to active bifunctional catalysts for electrochemical water-splitting, A. Indra, P. W. Menezes, I. Zaharieva, H. Dau, M. Driess, Journal of Materials Chemistry A 2020, 8, 2637–2643, 10.1039/C9TA09775A
Mechanistic studies of atomic layer deposition on oxidation catalysts – AlO and PO deposition, K. Knemeyer, M. Piernavieja Hermida, P. Ingale, J. Schmidt, J. Kröhnert, R. Naumann d’Alnoncourt, M. Driess, F. Rosowski, Physical Chemistry Chemical Physics 2020, 22, 17999–18006, 10.1039/D0CP02572K
A Systems Approach to a One‐Pot Electrochemical Wittig Olefination Avoiding the Use of Chemical Reductant or Sacrificial Electrode, B. Chakraborty, A. Kostenko, P. W. Menezes, M. Driess, Chemistry – A European Journal 2020, 26, 11829–11834, 10.1002/chem.202001654
An Isolable Bis(Silanone–Borane) Adduct, M. Luecke, E. Pens, S. Yao, M. Driess, Chemistry – A European Journal 2020, 26, 4500–4504, 10.1002/chem.202000235
Where silylene–silicon centres matter in the activation of small molecules, C. Shan, S. Yao, M. Driess, Chemical Society Reviews 2020, 49, 6733–6754, 10.1039/D0CS00815J
Beyond CO Reduction: Vistas on Electrochemical Reduction of Heavy Non-metal Oxides with Very Strong E—O Bonds (E = Si, P, S), B. Chakraborty, P. W. Menezes, M. Driess, Journal of the American Chemical Society 2020, 142, 14772–14788, 10.1021/jacs.0c05862
Enabling Iron‐Based Highly Effective Electrochemical Water‐Splitting and Selective Oxygenation of Organic Substrates through In Situ Surface Modification of Intermetallic Iron Stannide Precatalyst, B. Chakraborty, R. Beltrán‐Suito, J. N. Hausmann, S. Garai, M. Driess, P. W. Menezes, Advanced Energy Materials 2020, 10, 2001377–0, 10.1002/aenm.202001377
Immobilization of an Iridium Pincer Complex in a Microporous Polymer for Application in Room‐Temperature Gas Phase Catalysis, M. König, M. Rigo, N. Chaoui, T. Tran Ngoc, J. D. Epping, J. Schmidt, P. Pachfule, M. Ye, M. Trunk, J. F. Teichert, M. Drieß, A. Thomas, Angewandte Chemie International Edition 2020, 59, 19830–19834, 10.1002/anie.202004092
A bis(silylene)-stabilized diphosphorus compound and its reactivity as a monophosphorus anion transfer reagent, Y. Wang, T. Szilvási, S. Yao, M. Driess, Nature Chemistry 2020, 12, 801–807, 10.1038/s41557-020-0518-0
Novel, large area scalable polycrystalline Zn1-xCoxO films RF sputtered from a single mixed target for electrochemical water oxidation, J. Pfrommer, A. Steigert, C. Goebel, I. Lauermann, W. Calvet, R. Klenk, S. Mikhailov, A. Azarpira, S. Selve, M. Lublow, T. Schedel-Niedrig, M. Driess, International Journal of Hydrogen Energy 2020, 45, 9380–9385, 10.1016/j.ijhydene.2020.01.216
Cycloaddition Chemistry of a Silylene‐Nickel Complex toward Organic π‐Systems: From Reversibility to C−H Activation, T. J. Hadlington, A. Kostenko, M. Driess, Chemistry – A European Journal 2020, 26, 1958–1962, 10.1002/chem.202000009
Homocoupling of CO and isocyanide mediated by a , ′-bis(silylenyl)-substituted -carborane, Y. Xiong, S. Yao, T. Szilvási, A. Ruzicka, M. Driess, Chemical Communications 2020, 56, 747–750, 10.1039/C9CC08680C
Stannites – A New Promising Class of Durable Electrocatalysts for Efficient Water Oxidation, J. N. Hausmann, E. M. Heppke, R. Beltrán‐Suito, J. Schmidt, M. Mühlbauer, M. Lerch, P. W. Menezes, M. Driess, ChemCatChem 2020, 12, 1161–1168, 10.1002/cctc.201901705
Evaluation of Local Hybrid Functionals for Electric Properties: Dipole Moments and Static and Dynamic Polarizabilities, R. Grotjahn, G. J. Lauter, M. Haasler, M. Kaupp, The Journal of Physical Chemistry A 2020, 124, 8346–8358, 10.1021/acs.jpca.0c06939
Picometer Resolution Structure of the Coordination Sphere in the Metal-Binding Site in a Metalloprotein by NMR, A. Bertarello, L. Benda, K. J. Sanders, A. J. Pell, M. J. Knight, V. Pelmenschikov, L. Gonnelli, I. C. Felli, M. Kaupp, L. Emsley, R. Pierattelli, G. Pintacuda, Journal of the American Chemical Society 2020, 142, 16757–16765, 10.1021/jacs.0c07339
Validation of Local Hybrid Functionals for Excited States: Structures, Fluorescence, Phosphorescence, and Vibronic Spectra, R. Grotjahn, M. Kaupp, Journal of Chemical Theory and Computation 2020, 16, 5821–5834, 10.1021/acs.jctc.0c00520
Covalent vs Charge-Shift Nature of the Metal–Metal Bond in Transition Metal Complexes: A Unified Understanding, J. Joy, D. Danovich, M. Kaupp, S. Shaik, Journal of the American Chemical Society 2020, 142, 12277–12287, 10.1021/jacs.0c03957
Relativistic Heavy-Neighbor-Atom Effects on NMR Shifts: Concepts and Trends Across the Periodic Table, J. Vı́cha, J. Novotný, S. Komorovsky, M. Straka, M. Kaupp, R. Marek, Chemical Reviews 2020, 120, 7065–7103, 10.1021/acs.chemrev.9b00785
Ein neutrales 1,4‐Diborabenzol als π‐Ligand in Actinoidkomplexen, V. Paprocki, P. Hrobárik, K. L. M. Harriman, M. S. Luff, T. Kupfer, M. Kaupp, M. Murugesu, H. Braunschweig, Angewandte Chemie 2020, 132, 13209–13216, 10.1002/ange.202004501
Stable Actinide π Complexes of a Neutral 1,4‐Diborabenzene, V. Paprocki, P. Hrobárik, K. L. M. Harriman, M. S. Luff, T. Kupfer, M. Kaupp, M. Murugesu, H. Braunschweig, Angewandte Chemie International Edition 2020, 59, 13109–13115, 10.1002/anie.202004501
C–P vs C–H Bond Cleavage of Triphenylphosphine at Platinum(0): Mechanism of Formation, Reactivity, Redox Chemistry, and NMR Chemical Shift Calculations of a μ-Phosphanido Diplatinum(II) Platform, A. Berkefeld, M. Reimann, G. Hörner, M. Kaupp, H. Schubert, Organometallics 2020, 39, 443–452, 10.1021/acs.organomet.9b00807
Mercaptothiacalixarenes Steer 24 Copper(I) Centers to form a Hollow‐Sphere Structure Featuring Cu S Motifs with Exceptionally Short Cu⋅⋅⋅Cu Distances, N. Frank, A. Dallmann, B. Braun‐Cula, C. Herwig, C. Limberg, Angewandte Chemie International Edition 2020, 59, 6735–6739, 10.1002/anie.201915882
Routes to Heterotrinuclear Metal Siloxide Complexes for Cooperative Activation of O, M. L. Wind, S. Hoof, B. Braun-Cula, C. Herwig, C. Limberg, Inorganic Chemistry 2020, 59, 6866–6875, 10.1021/acs.inorgchem.0c00279
Selective Transformation of Nickel‐Bound Formate to CO or C−C Coupling Products Triggered by Deprotonation and Steered by Alkali‐Metal Ions, P. Zimmermann, D. Ar, M. Rößler, P. Holze, B. Cula, C. Herwig, C. Limberg, Angewandte Chemie International Edition 2020, 60, 2312–2321, 10.1002/anie.202010180
Versatile Coordination Behavior of the Asymmetric Bis(3‐mesityl‐pyrazol‐1‐yl)(5‐mesitylpyrazol‐1‐yl) Hydroborate Ligand towards Late 3 d M Ions, L. Müller, V. L. Nadurata, B. Cula, S. Hoof, C. Herwig, C. Limberg, European Journal of Inorganic Chemistry 2020, 2021, 71–85, 10.1002/ejic.202000895
Modular, Self-Assembling Metallaphotocatalyst for Cross-Couplings Using the Full Visible-Light Spectrum, S. Reischauer, V. Strauss, B. Pieber, ACS Catalysis 2020, 10, 13269–13274, 10.1021/acscatal.0c03950
Nickel on nitrogen-doped carbon pellets for continuous-flow hydrogenation of biomass-derived compounds in water, F. Brandi, M. Bäumel, V. Molinari, I. Shekova, I. Lauermann, T. Heil, M. Antonietti, M. Al-Naji, Green Chemistry 2020, 22, 2755–2766, 10.1039/c9gc03826d
Multi-Scale Analysis of Integrated C1 (CH4 and CO2) Utilization Catalytic Processes: Impacts of Catalysts Characteristics up to Industrial-Scale Process Flowsheeting, Part II: Techno-Economic Analysis of Integrated C1 Utilization Process Scenarios, H. R. Godini, M. Azadi, M. Khadivi, R. Schomäcker, F. Gallucci, G. Wozny, J. U. Repke, Catalysts 2020, 10, 488–0, 10.3390/catal10050488
How Reliable Is the Electrochemical Readout of MIP Sensors?, A. Yarman, F. W. Scheller, Sensors 2020, 20, 2677–0, 10.3390/s20092677
Noninvasive biosensors for diagnostic biomarkers, A. Yarman, S. Kurbanoglu, F. W. Scheller in Commercial Biosensors and their Applications (Hrsg.: Mustafa Kemal Sezginturk ), Elsevier, 2020, 167–181, ISBN: 9780128185926
B(C F ) -Catalyzed Hydrosilylation of Vinylcyclopropanes, P. W. Long, T. He, M. Oestreich, Organic Letters 2020, 22, 7383–7386, 10.1021/acs.orglett.0c02751
Silylium‐Ion‐Promoted (5+1) Cycloaddition of Aryl‐Substituted Vinylcyclopropanes and Hydrosilanes Involving Aryl Migration, T. He, G. Wang, V. Bonetti, H. F. T. Klare, M. Oestreich, Angewandte Chemie International Edition 2020, 59, 12186–12191, 10.1002/anie.202004320
Synthesis of a Counteranion‐Stabilized Bis(silylium) Ion, Q. Wu, A. Roy, G. Wang, E. Irran, H. F. T. Klare, M. Oestreich, Angewandte Chemie International Edition 2020, 59, 10523–10526, 10.1002/anie.202003799
The two CO-dehydrogenases of Thermococcus sp. AM4, M. Benvenuti, M. Meneghello, C. Guendon, A. Jacq-Bailly, J. H. Jeoung, H. Dobbek, C. Léger, V. Fourmond, S. Dementin, Biochimica et Biophysica Acta (BBA) - Bioenergetics 2020, 1861, 148188–0, 10.1016/j.bbabio.2020.148188
Double‐Cubane [8Fe9S] Clusters: A Novel Nitrogenase‐Related Cofactor in Biology, J. Jeoung, B. M. Martins, H. Dobbek, ChemBioChem 2020, 21, 1710–1716, 10.1002/cbic.202000016
Synergistic electroreduction of carbon dioxide to carbon monoxide on bimetallic layered conjugated metal-organic frameworks, H. Zhong, M. Ghorbani-Asl, K. H. Ly, J. Zhang, J. Ge, M. Wang, Z. Liao, D. Makarov, E. Zschech, E. Brunner, I. M. Weidinger, J. Zhang, A. V. Krasheninnikov, S. Kaskel, R. Dong, X. Feng, Nature Communications 2020, 11, 1–10, 10.1038/s41467-020-15141-y
Electrolysis of low-grade and saline surface water, W. Tong, M. Forster, F. Dionigi, S. Dresp, R. Sadeghi Erami, P. Strasser, A. J. Cowan, P. Farràs, Nature Energy 2020, 5, 367–377, 10.1038/s41560-020-0550-8
P-block single-metal-site tin/nitrogen-doped carbon fuel cell cathode catalyst for oxygen reduction reaction, F. Luo, A. Roy, L. Silvioli, D. A. Cullen, A. Zitolo, M. T. Sougrati, I. C. Oguz, T. Mineva, D. Teschner, S. Wagner, J. Wen, F. Dionigi, U. I. Kramm, J. Rossmeisl, F. Jaouen, P. Strasser, nature materials 2020, 19, 1215–1223, 10.1038/s41563-020-0717-5
Electrocatalytic CO Reduction on CuO Nanocubes: Tracking the Evolution of Chemical State, Geometric Structure, and Catalytic Selectivity using Operando Spectroscopy, T. Möller, F. Scholten, T. N. Thanh, I. Sinev, J. Timoshenko, X. Wang, Z. Jovanov, M. Gliech, B. Roldan Cuenya, A. S. Varela, P. Strasser, Angewandte Chemie International Edition 2020, 59, 17974–17983, 10.1002/anie.202007136
Electrochemical Approaches toward CO Capture and Concentration, S. E. Renfrew, D. E. Starr, P. Strasser, ACS Catalysis 2020, 10, 13058–13074, 10.1021/acscatal.0c03639
Confinement of Cobalt Species in Mesoporous N-Doped Carbons and the Impact on Nitroarene Hydrogenation, R. L. Oliveira, M. C. Ben Ghorbel, S. Praetz, D. Meiling, C. Schlesiger, R. Schomäcker, A. Thomas, ACS Sustainable Chemistry & Engineering 2020, 8, 11171–11182, 10.1021/acssuschemeng.0c02365
Hydrogen Development, U. P. Apfel, W. Weigand, M. Horch, I. Zebger, O. Lenz, T. Fujishiro in Bioorganometallic Chemistry (Hrsg.: Wolfgang Weigand, Ulf-Peter Apfel), De Gruyter, 2020, 13–136, ISBN: 9783110496505
Immobilized dye-decolorizing peroxidase (DyP) and directed evolution variants for hydrogen peroxide biosensing, C. Barbosa, C. M. Silveira, D. Silva, V. Brissos, P. Hildebrandt, L. O. Martins, S. Todorovic, Biosensors and Bioelectronics 2020, 153, 112055–0, 10.1016/j.bios.2020.112055
Temperature Dependence of Structural Dynamics at the Catalytic Cofactor of [FeFe]-hydrogenase, S. T. Stripp, S. Mebs, M. Haumann, Inorganic Chemistry 2020, 59, 16474–16488, 10.1021/acs.inorgchem.0c02316
QM/MM computations reveal details of the acetyl-CoA synthase catalytic center, N. Elghobashi-Meinhardt, D. Tombolelli, M. A. Mroginski, Biochimica et Biophysica Acta (BBA) - General Subjects 2020, 1864, 129579–0, 10.1016/j.bbagen.2020.129579
Key role of chemistry versus bias in electrocatalytic oxygen evolution, H. N. Nong, L. J. Falling, A. Bergmann, M. Klingenhof, H. P. Tran, C. Spöri, R. Mom, J. Timoshenko, G. Zichittella, A. Knop-Gericke, S. Piccinin, J. Pérez-Ramírez, B. Roldan Cuenya, R. Schlögl, P. Strasser, D. Teschner, T. E. Jones, Nature 2020, 587, 408–413, 10.1038/s41586-020-2908-2
Structural Complexity and Plasticity of Signaling Regulation at the Melanocortin-4 Receptor, G. Kleinau, N. A. Heyder, Y. X. Tao, P. Scheerer, International Journal of Molecular Sciences 2020, 21, 5728–0, 10.3390/ijms21165728
An Engineered Strain with Synthetic Metabolism for in‐Cell Production of Translationally Active Methionine Derivatives, C. J. Schipp, Y. Ma, A. Al‐Shameri, F. D'Alessio, P. Neubauer, R. Contestabile, N. Budisa, M. L. di Salvo, ChemBioChem 2020, 21, 3525–3538, 10.1002/cbic.202000257
Thermodynamic Reaction Control of Nucleoside Phosphorolysis, F. Kaspar, R. T. Giessmann, P. Neubauer, A. Wagner, M. Gimpel, Advanced Synthesis & Catalysis 2020, 362, 867–876, 10.1002/adsc.201901230
General Principles for Yield Optimization of Nucleoside Phosphorylase‐Catalyzed Transglycosylations, F. Kaspar, R. T. Giessmann, K. F. Hellendahl, P. Neubauer, A. Wagner, M. Gimpel, ChemBioChem 2020, 21, 1428–1432, 10.1002/cbic.201900740
Efficient Biocatalytic Synthesis of Dihalogenated Purine Nucleoside Analogues Applying Thermodynamic Calculations, H. Yehia, S. Westarp, V. Röhrs, F. Kaspar, R. T. Giessmann, H. F. T. Klare, K. Paulick, P. Neubauer, J. Kurreck, A. Wagner, Molecules 2020, 25, 934–0, 10.3390/molecules25040934
Spectral Unmixing‐Based Reaction Monitoring of Transformations between Nucleosides and Nucleobases, F. Kaspar, R. T. Giessmann, S. Westarp, K. F. Hellendahl, N. Krausch, I. Thiele, M. C. Walczak, P. Neubauer, A. Wagner, ChemBioChem 2020, 21, 2604–2610, 10.1002/cbic.202000204
observation of pH change during water splitting in neutral pH conditions: impact of natural convection driven by buoyancy effects, K. Obata, R. van de Krol, M. Schwarze, R. Schomäcker, F. F. Abdi, Energy & Environmental Science 2020, 13, 5104–5116, 10.1039/d0ee01760d
Elucidation of Cooperativity in CO Reduction Using a Xanthene-Bridged Bimetallic Rhenium(I) Complex, R. Giereth, P. Lang, E. McQueen, X. Meißner, B. Braun-Cula, C. Marchfelder, M. Obermeier, M. Schwalbe, S. Tschierlei, ACS Catalysis 2020, 11, 390–403, 10.1021/acscatal.0c04314
Matters of class: coming of age of class III and IV lanthipeptides, J. D. Hegemann, R. D. Süssmuth, RSC Chemical Biology 2020, 1, 110–127, 10.1039/d0cb00073f
Current limits of structural biology: The transient interaction between cytochrome c and photosystem I, A. Kölsch, C. Radon, M. Golub, A. Baumert, J. Bürger, T. Mielke, F. Lisdat, A. Feoktystov, J. Pieper, A. Zouni, P. Wendler, Current Research in Structural Biology 2020, 2, 171–179, 10.1016/j.crstbi.2020.08.003
H2 as a fuel for flavin- and H2O2-dependent biocatalytic reactions, A. Al-Shameri, S. J. P. Willot, C. E. Paul, F. Hollmann, L. Lauterbach, Chemical Communications 2020, 56, 9667–9670, 10.1039/D0CC03229H
Powering Artificial Enzymatic Cascades with Electrical Energy, A. Al‐Shameri, M. Petrich, K. junge Puring, U. Apfel, B. M. Nestl, L. Lauterbach, Angewandte Chemie International Edition 2020, 59, 10929–10933, 10.1002/anie.202001302
Kristallstruktur und Spektroskopie offenbaren einen Schwefel‐Liganden am aktiven Zentrum einer O ‐stabilen [FeFe]‐Hydrogenase, P. Rodríguez‐Maciá, L. M. Galle, R. Bjornsson, C. Lorent, I. Zebger, Y. Yoda, S. P. Cramer, S. DeBeer, I. Span, J. A. Birrell, Angewandte Chemie 2020, 132, 16930–16939, 10.1002/ange.202005208